Metal Catalyzed Reductive C–C Bond Formation: A Departure by John Montgomery, Grant J. Sormunen (auth.), Michael J.

By John Montgomery, Grant J. Sormunen (auth.), Michael J. Krische (eds.)

J. Montgomery, G.J. Sormunen: Nickel-Catalyzed Reductive Couplings of Aldehydes and Alkynes.-

A. Gansäuer, J. Justicia, C.-A. Fan, D. Worgull, F. Piestert: Reductive C-C Bond Formation after Epoxide beginning through Electron Transfer.-

T. Hirao: Catalytic Reductive Coupling of Carbonyl Compounds - The Pinacol Coupling response and Beyond.-

H. Iida, M.J. Krische: Catalytic Reductive Coupling of Alkenes and Alkynes to Carbonyl Compounds and Imines Mediated through Hydrogen.-

H. Nishiyama, T. Shiomi: Reductive Aldol, Michael and Mannich Reactions.-

B. Breit: contemporary Advances in Alkene Hydroformylation.-

M. Kimura, Y. Tamaru: Nickel-Catalyzed Reductive Coupling of Dienes and Carbonyl Compounds.-

R.D. Broene: Reductive Coupling of Unactivated Alkenes and Alkynes

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Metal Catalyzed Reductive C–C Bond Formation: A Departure from Preformed Organometallic Reagents

J. Montgomery, G. J. Sormunen: Nickel-Catalyzed Reductive Couplings of Aldehydes and Alkynes. -A. Gansäuer, J. Justicia, C. -A. Fan, D. Worgull, F. Piestert: Reductive C-C Bond Formation after Epoxide beginning through Electron move. -T. Hirao: Catalytic Reductive Coupling of Carbonyl Compounds - The Pinacol Coupling response and past.

Extra resources for Metal Catalyzed Reductive C–C Bond Formation: A Departure from Preformed Organometallic Reagents

Sample text

34 34 34 35 45 45 47 Conclusion . . . . . . . . . . . . . . . . . . 48 References . . . . . . . . . . . . . . . . . . . . 3 Formation of C–C Bonds by Intermolecular Stoichiometric Reactions . . . . . . Catalytic Reactions . . . . . . . Polymerizations . . . . . . . . Addition . . . . . . . . . 2 Cyclizations . . . . . .

This amply demonstrates the flexibility of their catalytic protocol. It should be noted that by this elegant semisynthetic approach the side-products of biosynthesis can be efficiently obtained. Scheme 24 Oltra’s and Cuerva’s transannular cyclizations Later the same group reported the application of their method in the synthesis of a number of natural products from simple starting materials such as epoxygeranyl acetate, ketals of epoxygeranylacetone or the epoxy acetate of geranyl geraniol as shown in Scheme 25.

Structure of the Reagent and Mechanism of Epoxide Opening . . . . 27 27 28 Formation of C–C Double Bonds by Epoxide Deoxygenation and Epoxide Dimerization . . . . . . . . . . . . . . 29 . . . . . . . . . . . . . . . . . . . . . . 31 31 33 34 . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 34 34 34 35 45 45 47 Conclusion . . . . . . . . . . . .

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